INTENSE HIGH HARMONIC GENERATION IN FULLERENE MOLECULE C180
- 作者: Avetisyan G.K.1, Kazaryan A.G.1, Matevosyan G.G.2, Mkrtchyan G.F.1
-
隶属关系:
- Centre of Strong Fields Physics at Physics Research Institute, Yerevan State University
- Institute of Radiophysics and Electronics NAS RA
- 期: 卷 165, 编号 1 (2024)
- 页面: 25-31
- 栏目: Articles
- URL: https://ogarev-online.ru/0044-4510/article/view/256894
- DOI: https://doi.org/10.31857/S0044451024010036
- ID: 256894
如何引用文章
详细
Investigation of high‑order harmonic generation (HHG) in the large fullerene C180 molecule under intense laser field is presented. To model the С180 molecule and its interaction with the laser field, we employ the tight‑binding mean‑field approach. Our detailed analysis of the HHG power spectrum reveals the multiphoton resonant nature of harmonic generation, shedding light on the underlying quantum processes involved. We examine the dependence of cutoff harmonics on both laser intensity and frequency, providing valuable insights into the optimal conditions for enhancing HHG in C180. We demonstrate that the C180 molecule exhibits a significantly stronger high harmonic intensity compared to the more widely studied C60 fullerene.
作者简介
G. Avetisyan
Centre of Strong Fields Physics at Physics Research Institute, Yerevan State University
Email: amarkos@ysu.am
亚美尼亚, 0025, Yerevan
A. Kazaryan
Centre of Strong Fields Physics at Physics Research Institute, Yerevan State University
Email: amarkos@ysu.am
亚美尼亚, 0025, Yerevan
G. Matevosyan
Institute of Radiophysics and Electronics NAS RA
Email: amarkos@ysu.am
亚美尼亚, 0203, Ashtarak
G. Mkrtchyan
Centre of Strong Fields Physics at Physics Research Institute, Yerevan State University
编辑信件的主要联系方式.
Email: amarkos@ysu.am
亚美尼亚, 0025, Yerevan
参考
- P. B. Corkum, Phys. Rev. Lett. 71, 1994 (1993).
- M. Lewenstein, P. Balcou, M. Y. Ivanov et al., Phys. Rev. A 49, 2117 (1994).
- H. K. Avetissian, Relativistic Nonlinear Electrodynamics: The QED Vacuum and Matter in Super- Strong Radiation Fields, Springer, New York (2015).
- P. B. Corkum and F. Krausz, Nature Phys. 3, 381 (2007).
- F. Krausz and M. Ivanov, Rev. Mod. Phys. 81, 163 (2009).
- E. H. Falcao and F. Wudl, J. Chem. Technol. Biotechnol. 82, 524 (2007).
- S. K. Tiwari, V. Kumar, A. Huczko, et al., Critical Rev. Sol. State and Mater. Sci. 41, 257 (2016).
- R. E. Smalley, Rev. Mod. Phys. 69, 723 (1997).
- H. W. Kroto, J. R. Heath, S. C. O’Brien et al., Nature 318, 162 (1985).
- H. Kroto and K. McKay, Nature 331, 328 (1988).
- D. York, J. P. Lu, and W. Yang, Phys. Rev. B 49, 8526 (1994).
- G. E. Scuseria, Chem. Phys. Lett. 243, 193 (1995).
- G. E. Scuseria, Science 271, 942 (1996).
- S. Itoh, P. Ordejon, D. A. Drabold, and R. M. Martin, Phys. Rev. B 53, 2132 (1996).
- C. H. Xu and G. E. Scuseria, Chem. Phys. Lett. 262, 219 (1996).
- P. W. Dunk, N. K. Kaiser, C. L. Hendrickson et al., Nature Commun. 3, 855 (2012).
- J. W. Martin, G. J. McIntosh, R. Aru et al., Carbon 125, 132 (2017).
- S. Wang, Q. Chang, G. Zhang et al., Front. Chem. 8, 607712 (2020).
- E. Ghavanloo, H. Rai-Tabar, A. Kausar et al., Phys. Rep. 996, 1 (2023).
- T.D. Donnelly, T. Ditmire, K. Neuman et al., Phys. Rev. Lett. 76, 2472 (1996).
- C. Vozzi, M. Nisoli, J. Caumes et al., Appl. Phys. Lett. 86 (2005).
- O. Smirnova, Y. Mairesse, S. Patchkovski et al., Nature 460, 972 (2009).
- Б.Р. Авчян, А. Г. Казарян, К. А. Сарг- сян, Х. В. Седракян, ЖЭТФ 161, 155 (2022).
- B.R. Avchyan, A.G. Ghazaryan, S.S. Israelyan, and K. V. Sedrakian, J. Nanophot. 16, 036001 (2022).
- Б.Р. Авчян, А. Г. Казарян, К. А. Саргсян, Х. В. Седракян, Письма в ЖЭТФ 116, 426 (2022).
- S. Gnawali, R. Ghimire, K. R. Maga et al., Phys. Rev. B 106, 075149 (2022).
- R. Ganeev, L.E. Bom, J. Abdul-Hadi et al., Phys. Rev. Lett. 102, 013903 (2009).
- R. Ganeev, L.E. Bom, M. Wong et al., Phys. Rev. A 80, 043808 (2009).
- G.P. Zhang, Phys. Rev. Lett. 95, 047401 (2005).
- G.P. Zhang and T. F. George, Phys. Rev. A 74, 023811 (2006).
- G.P. Zhang and Y.H. Bai, Phys. Rev. B 101, 081412(R) (2020).
- H.K. Avetissian, A.G. Ghazaryan, and G.F. Mkrtchian, Phys. Rev. B 104, 125436 (2021).
- H.K. Avetissian, S. Sukiasyan, H.H. Matevosyan, and G.F. Mkrtchian, Results Phys. 53, 106951 (2003), https://doi.org/10.1016/j.rinp.2023.106951, arXiv:2304.04208 (2023).
- R.L. Martin and J.P. Ritchie, Phys. Rev. B 48, 4845 (1993).
- G. Zhang, Phys. Rev. B 56, 9189 (1997).
- P. W. Fowler and D. E. Manolopoulos, An Atlas of Fullerenes, Courier Corporation, New York (2007).
- P. Schwerdtfeger, L. Wirz, and J. Avery, J. Comput. Chem. 34, 1508 (2013).
- G.P. Zhang, M.S. Si, M. Murakami et al., Nature Commun. 9, 3031 (2018).
补充文件
