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Том 124, № 3 (2018)

Spectroscopy of Atoms and Molecules

On Precision Measurement of the Frequency of the 11S–23S Forbidden Transition of a Helium Atom

Baklanov E., Tai’chenachev A.

Аннотация

The possibility is demonstrated of a precision frequency measurement for the 11S0−23S1 forbidden transition (at 62.6 nm) of a helium atom using the stimulated Raman scattering method. The 11S0 singlet state is the ground state of 4He, while the metastable 23S1 state has the lowest energy in the triplet part of the spectrum (4He*). The transition has a very small natural width, which allows us to consider it as a possible reference for creation of a frequency standard in the vacuum ultraviolet region.

Optics and Spectroscopy. 2018;124(3):285-288
pages 285-288 views

Condensed-Matter Spectroscopy

Determining the Size of Pores in a Partially Transparent Ceramics from Total-Reflection Spectra

Mironov R., Zabezhailov M., Georgiu I., Cherepanov V., Rusin M.

Аннотация

A technique is proposed for determining the pore-size distribution based on measuring the dependence of total reflectance in the domain of partial transparency of a material. An assumption about equality of scattering-coefficient spectra determined by solving the inverse radiation transfer problem and by theoretical calculation with the Mie theory is used. The technique is applied to studying a quartz ceramics. The poresize distribution is also determined using mercury and gas porosimetry. All three methods are shown to produce close results for pores with diameters of <180 nm, which occupy ~90% of the void volume. In the domain of pore dimensions of >180 nm, the methods show differences that might be related to both specific procedural features and the structural properties of ceramics. The spectral-scattering method has a number of advantages over traditional porosimetry, and it can be viewed as a routine industrial technique.

Optics and Spectroscopy. 2018;124(3):289-297
pages 289-297 views

Spectral-Luminescence Properties of Europium(III) Compounds with Two Different β-Diketones

Kalinovskaya I.

Аннотация

Complex luminescent mixed-ligand compounds of europium(III) with two different β-diketones have been synthesized. Spectral-luminescence properties of complex europium(III) compounds have been investigated. The copresence of two different β-diketones in the europium(III) coordination sphere results in expansion of the spectral-absorption range, as well as in luminescence-intensity growth.

Optics and Spectroscopy. 2018;124(3):298-301
pages 298-301 views

Optical Characteristics of Pyrolytic Carbon in the Vicinity of the E1u Vibrational Mode Calculated within the Framework of the Effective-Medium Model

Bekhterev A., Ryzhov A.

Аннотация

Spectral optical constants of pyrolytic carbon in the region of activity of the E1u vibrational mode are calculated within the framework of the effective-medium approach in the Bruggeman approximation. It is demonstrated that the number, position, half-width, and relative intensity of the selective-absorption bands in the IR absorption spectrum of pyrolytic carbon are the independent of porosity of the original absorbing object.

Optics and Spectroscopy. 2018;124(3):302-306
pages 302-306 views

Anti-Stokes Luminescence in LiYF4:Ho3+, Yb3+ Ceramics Excited at 1.93 μm

Savikin A., Perunin I., Kurashkin S., Budruev A., Grishin I.

Аннотация

Conversion of IR radiation of a Tm:YAP laser with a wavelength of 1930 nm into visible light by ceramics of composition LiY(1–x–y) HoxYby, where х = 1–5 mol % and y = 0–15 mol %, is demonstrated. It is shown that the threshold power density of IR light visualization decreases with increasing concentration of Ho3+ ions, while additional doping of ceramic samples with Yb3+ ions changes the anti-Stokes luminescence spectrum. The threshold power density of visualization of the Tm:YAP laser radiation decreases with increasing concentration of holmium ions and is Ithr ≈ 0.8 W cm–2 in the samples of composition LiYF4:5%Ho3+–15%Yb3+.

Optics and Spectroscopy. 2018;124(3):307-309
pages 307-309 views

The Influence of the Direction of External Magnetic Field on the Band Structure of Magneto-Photonic Crystals

Gevorgyan A., Golik S., Gevorgyan T.

Аннотация

Specific features of the energy-band structure of magneto-photonic crystals have been studied. The problem of the propagation of light through a finite layer of a magneto-photonic crystal has been solved by the modified Ambartsumyan layer-summation method. The effect of the direction of an external magnetic field on the band structure has been studied in detail and shown to alter the number of forbidden bands, change the frequency widths of these bands, and modify their polarization-related properties. Such systems have been shown to possess four eigenpolarizations.

Optics and Spectroscopy. 2018;124(3):310-318
pages 310-318 views

Enhancement of Fluorescence and Raman Scattering in Cyanine-Dye Molecules on the Surface of Silicon-Coated Silver Nanoparticles

Kamalieva A., Toropov N., Bogdanov K., Vartanyan T.

Аннотация

A method of formation of a composite structure based on silver nanoparticles and a thin protective silicon film (AgNPs/Si) is developed. Enhancement of the fluorescence and Raman scattering in cyaninedye molecules deposited onto the formed nanostructure is observed. The optical properties and morphology stability of particles that are in contact with cyanine-dye solutions in organic solvents are studied. It is shown that the AgNPs/Si composite structure can be multiply used as an SERS-active surface.

Optics and Spectroscopy. 2018;124(3):319-322
pages 319-322 views

Radiothermoluminescence of Oxide Nanostructures on Surfaces of Radiation-Oxidized Aluminum and Beryllium

Gadzhieva N., Magerramov A.

Аннотация

The formation dynamics of oxide nanostructures on surfaces of oxidized aluminum and beryllium with water at room temperature and under radiation action has been studied by the radiothermoluminescence method. The role of intermediate surface active particles in the dynamics of changes of the oxidation process of aluminum and beryllium in an absorbed dose range of 0.5–120 kGy has been considered. It is established that, when nanostructure films are formed, molecular oxygen and other oxygen-containing ion-radical groups generated by γ irradiation play the main role. The radiation-oxidation kinetics of aluminum and beryllium is studied, and their chemisorption passivation is revealed. A possible mechanism of this process is discussed.

Optics and Spectroscopy. 2018;124(3):323-327
pages 323-327 views

The Composition of Intermediate Products of the Thermal Decomposition of (NH4)2ZrF6 to ZrO2 from Vibrational-Spectroscopy Data

Voit E., Didenko N., Gaivoronskaya K.

Аннотация

Thermal decomposition of (NH4)2ZrF6 resulting in ZrO2 formation within the temperature range of 20°–750°С has been investigated by means of thermal and X-ray diffraction analysis and IR and Raman spectroscopy. It has been established that thermolysis proceeds in six stages. The vibrational-spectroscopy data for the intermediate products of thermal decomposition have been obtained, systematized, and summarized.

Optics and Spectroscopy. 2018;124(3):328-336
pages 328-336 views

Nonlinear and Quantum Optics

A Novel Approach to Realize of All Optical Frequency Encoded Dibit Based XOR and XNOR Logic Gates Using Optical Switches with Simulated Verification

Ghosh B., Hazra S., Haldar N., Roy D., Patra S., Swarnakar J., Sarkar P., Mukhopadhyay S.

Аннотация

Since last few decades optics has already proved its strong potentiality for conducting parallel logic, arithmetic and algebraic operations due to its super-fast speed in communication and computation. So many different logical and sequential operations using all optical frequency encoding technique have been proposed by several authors. Here, we have keened out all optical dibit representation technique, which has the advantages of high speed operation as well as reducing the bit error problem. Exploiting this phenomenon, we have proposed all optical frequency encoded dibit based XOR and XNOR logic gates using the optical switches like add/drop multiplexer (ADM) and reflected semiconductor optical amplifier (RSOA). Also the operations of these gates have been verified through proper simulation using MATLAB (R2008a).

Optics and Spectroscopy. 2018;124(3):337-342
pages 337-342 views

A Fiber-Optic System Generating Pulses of High Spectral Density

Abramov A., Zolotovskii I., Korobko D., Fotiadi A.

Аннотация

A cascade fiber-optic system that generates pulses of high spectral density by using the effect of nonlinear spectral compression is proposed. It is demonstrated that the shape of the pulse envelope substantially influences the degree of compression of its spectrum. In so doing, maximum compression is achieved for parabolic pulses. The cascade system includes an optical fiber exhibiting normal dispersion that decreases along the fiber length, thereby ensuring that the pulse envelope evolves toward a parabolic shape, along with diffraction gratings and a fiber spectral compressor. Based on computer simulation, we determined parameters of cascade elements leading to maximum spectral density of radiation originating from a subpicosecond laser pulse of medium energy.

Optics and Spectroscopy. 2018;124(3):343-348
pages 343-348 views

Physical Optics

Coherence Volume of an Optical Wave Field with Broad Frequency and Angular Spectra

Lyakin D., Mysina N., Ryabukho V.

Аннотация

We consider the sizes of a region in a three-dimensional space in which an optical wave field excites mutually coherent perturbations. We discuss the conditions under which the length of this region along the direction of propagation of the wave field and, correspondingly, its volume are determined either by the width of the frequency spectrum of the field or by the width of its angular spectrum, or by the parameters of these spectra simultaneously. We obtain expressions for estimating extremely small values of the coherence volume of the fields with a broad frequency spectrum and an extremely broad angular spectrum. Using the notion of instantaneous speckle-modulation of the wave field, we give a physical interpretation to the occurrence of a limited coherence volume of the field. The length of the spatiotemporal coherence region in which mutually coherent perturbations occur at different times is determined. The coherence volume of a wave field that illuminates an object in high-resolution microscopy with frequency broadband light is considered. The conditions for the dominant influence of the angular or frequency spectra on the longitudinal length of the coherence region are given, and the conditions for the influence of the frequency spectrum width on the transverse coherence of the wave field are examined. We show that, when using fields with broad and ultrabroad spectra in high-resolution microscopy, this influence should be taken into account.

Optics and Spectroscopy. 2018;124(3):349-359
pages 349-359 views

Linear Transformation of the Polarization Modes in Coiled Optical Spun-Fibers with Strong Unperturbed Linear Birefringence. I. Nonresonant Transformation

Malykin G., Pozdnyakova V.

Аннотация

A linear transformation of orthogonal polarization modes in coiled optical spun-fibers with strong unperturbed linear birefringence, which causes the emergence of the dependences of the integrated elliptical birefringence and the ellipticity and azimuth of the major axis of the ellipse, as well as the polarization state of radiation (PSR), on the length of optical fiber has been considered. Optical spun-fibers are subjected to a strong mechanical twisting, which is frozen into the structure of the optical fiber upon cooling, in the process of being drawn out from the workpiece. Since the values of the local polarization parameters of coiled spunwaveguides vary according to a rather complex law, the calculations were carried out by numerical modeling of the parameters of the Jones matrices. Since the rotation speed of the axes of the birefringence is constant on a relatively short segment of a coiled optical spun-fiber in the accompanying torsion (helical) coordinate system, the so-called “Ginzburg helical polarization modes” (GHPMs)—two mutually orthogonal ellipses with the opposite directions of traversal, the axis of which rotate relative to the fixed coordinate system uniformly and unidirectionally—are approximately the local normal polarization modes of such optical fiber. It has been shown that, despite the fact that the unperturbed linear birefringence of the spun-fibers significantly exceeds the linear birefringence, which is caused by the winding on a coil, the integral birefringence of an extended segment of such a fiber coincides in order of magnitude with the linear birefringence, which is caused by the winding on the coil, and the integral polarization modes tend asymptotically to circular ones. It has been also shown that the values of the circular birefringence of twisted single-mode fibers, which were calculated in a nonrotating and torsion helical coordinate systems, differ significantly. It has been shown that the polarization phenomena occur in the process of linear transformation of local polarization modes, which lead to small quasi-harmonic oscillations of the birefringence integral parameters of the optical spun-fibers, which depend on their length, and the period of these oscillations is approximately equal to half of the effective period of polarization beating.

Optics and Spectroscopy. 2018;124(3):360-372
pages 360-372 views

Holography

The Current Status of the Development of Light-Sensitive Media for Holography (a Review)

Barachevsky V.

Аннотация

The results of studies that have been performed over the last decade in the field of development of silver halide and nonsilver holographic recording media of organic and inorganic origin are analyzed. It is shown that previously developed materials mainly allow the development of holographic investigations. Among irreversible materials, considerable progress has been made in improving the characteristics of photopolymerizable recording media, which has allowed their use in color image holography and 3D optical archive-type memory, as well as for fabricating holographic optical elements. In the field of improving the properties of reversible holographic recording media, practically significant results have been obtained for the creation of photoanisotropic materials based on azo dyes experiencing cis–trans photoisomerization, which allow the recording of polarization holograms. The needs of dynamic holography have been satisfied by lightsensitive doped inorganic crystals and polymer layers that have been created with nonlinear optical properties.

Optics and Spectroscopy. 2018;124(3):373-407
pages 373-407 views

The Transfer of a Holographic Structure from Dihromated Gelatin Layers on a Polymethylmethacrylate Substrate

Ganzherli N., Gulyaev S., Maurer I., Khazvalieva D.

Аннотация

The possibility of the transfer of a holographic structure that was originally registered on layers of dichromated gelatin (DCG) onto a substrate material of polymethylmethacrylate (PMMA) has been shown. The use of a selective destructive effect of short-wave UV radiation with a wavelength that is less than 270 nm is the basis of the mechanism of formation of secondary relief-phase holographic structure on the surface of PMMA. The optimization of processing modes and selection of developing compositions which are based on isopropanol and methylisobutylketone (MIBK) have been carried out, which made it possible to create reliefphase holographic gratings with high diffraction efficiency (DE) of about 25% and the maximum depth of the surface relief of the order of 1 μm on the substrates of PMMA.

Optics and Spectroscopy. 2018;124(3):408-411
pages 408-411 views

Lasers and their Applications

Optoacoustic Effects in Pentaerythritol Tetranitrate with Ultrafine Aluminum-Particle Inclusions under Pulsed-Laser Action

Aduev B., Nurmukhametov D., Belokurov G., Nelyubina N., Tupitsyn A.

Аннотация

Results of studying optoacoustic characteristics of pentaerythritol tetranitrate (PETN) specimens with inclusions of ultrafine aluminum particles (100 nm) are presented. Regularities of the increase of extinction coefficient kef and signal amplitude U on a piezodetector by increasing laser-pulse fluence H have been established. Estimates have been made, and it has been concluded that, during a laser pulse, heating of aluminum inclusions and a shell surrounding it occurs up to a gasification temperature and appear craters on a specimen’s surface appear at H > 0.1 J/cm2.

Optics and Spectroscopy. 2018;124(3):412-417
pages 412-417 views

Dynamics of a Wave Packet of Whispering-Gallery-Mode Type in an Optical Waveguide in the Presence of a Traveling Refractive-Index Wave

Zolotovskii I., Korobko D., Mironov P., Sementsov D., Fotiadi A., Yavtushenko M.

Аннотация

It is demonstrated that strong ultrafast modulation of a tunneling wave packet of the whispering-gallery-mode type can be implemented in a cylindrical optical waveguide exhibiting spatiotemporal inhomogeneity induced by a travelling refractive-index wave. The corresponding optical waveguides can be used for efficient generation of picosecond and subpicosecond laser pulses.

Optics and Spectroscopy. 2018;124(3):418-423
pages 418-423 views

Geometrical and Applied Optics

Diffraction Dilatometry of Polymethacrylate at Low Temperatures

Farrakhov B., Fattakhov Y., Galyautdinov M., Stepanov A.

Аннотация

The linear thermal-expansion coefficient of polymethacrylate is measured in the temperature range from–194 to 0°С. A dilatometric study was performed using optical diffraction.

Optics and Spectroscopy. 2018;124(3):424-427
pages 424-427 views

Wide-Aperture Aspheric Optics for Formation of Subwavelength Caustics of a Terahertz Electromagnetic-Radiation Beam

Chernomyrdin N., Shchadko A., Lebedev S., Spektor I., Tolstoguzov V., Kucheryavenko A., Malakhov K., Komandin G., Gorelik V., Zaytsev K.

Аннотация

A wide-aperture aspheric lens for focusing a terahertz electromagnetic-radiation beam in a circle of the subwavelength size is proposed. The calculation of the lens and the estimation of size of created caustic were carried out using computational methods of geometric optics and electrodynamics. The lens is made of high-density polyethylene with the help of a turning machine. For experimental estimation of the spatial resolution provided by the lens, a THz imaging system based on raster scanning of the object’s surface was created. The imaging system was used in combination with wide-aperture THz optics to record images of the streak plates with different spatial frequencies. Analysis of the experimental data showed that the aspheric lens allows the resolution of two objects spaced at a distance of 0.95λ, providing contrast of 15%. The proposed THz optics is superior to classical THz spherical lenses and off-axis parabolic mirrors, greatly expanding the capabilities of THz-spectroscopy methods and imaging.

Optics and Spectroscopy. 2018;124(3):428-436
pages 428-436 views

Analysis of Fringe Field Formed Inside LDA Measurement Volume Using Compact Two Hololens Imaging Systems

Ghosh A., Nirala A., Yadav H.

Аннотация

We have designed and fabricated four LDA optical setups consisting of aberration compensated four different compact two hololens imaging systems. We have experimentally investigated and realized a hololens recording geometry which is interferogram of converging spherical wavefront with mutually coherent planar wavefront. Proposed real time monitoring and actual fringe field analysis techniques allow complete characterizations of fringes formed at measurement volume and permit to evaluate beam quality, alignment and fringe uniformity with greater precision. After experimentally analyzing the fringes formed at measurement volume by all four imaging systems, it is found that fringes obtained using compact two hololens imaging systems get improved both qualitatively and quantitatively compared to that obtained using conventional imaging system. Results indicate qualitative improvement of non-uniformity in fringe thickness and micro intensity variations perpendicular to the fringes, and quantitative improvement of 39.25% in overall average normalized standard deviations of fringe width formed by compact two hololens imaging systems compare to that of conventional imaging system.

Optics and Spectroscopy. 2018;124(3):437-449
pages 437-449 views

Erratum

Erratum to: “Time-Harmonic Gaussian Beams: Exact Solutions of the Helmhotz Equation in Free Space”

Kiselev A.

Аннотация

Equation (25) should be read as follows:

Optics and Spectroscopy. 2018;124(3):450-450
pages 450-450 views