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Preparation, Structure, and Dielectric and Nonlinear Optical Properties of (K0.5Na0.5)NbO3–BaZrO3 Ceramics

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1. Title Title of document Preparation, Structure, and Dielectric and Nonlinear Optical Properties of (K0.5Na0.5)NbO3–BaZrO3 Ceramics
2. Creator Author's name, affiliation, country G. M. Kaleva; Semenov Federal Research Center for Chemical Physics, Russian Academy of Sciences, 119991, Moscow, Russia
2. Creator Author's name, affiliation, country E. D. Politova; Semenov Federal Research Center for Chemical Physics, Russian Academy of Sciences, 119991, Moscow, Russia
2. Creator Author's name, affiliation, country S. A. Ivanov; Semenov Federal Research Center for Chemical Physics, Russian Academy of Sciences, 119991, Moscow, Russia; Moscow State University, 119991, Moscow, Russia
2. Creator Author's name, affiliation, country A. V. Mosunov; Moscow State University, 119991, Moscow, Russia
2. Creator Author's name, affiliation, country S. Yu. Stefanovich; Moscow State University, 119991, Moscow, Russia
2. Creator Author's name, affiliation, country N. V. Sadovskaya; Shubnikov Institute of Crystallography, Crystallography and Photonics Federal Scientific Research Center, Russian Academy of Sciences, 119333, Moscow, Russia
3. Subject Discipline(s)
3. Subject Keyword(s) potassium sodium niobate; perovskite structure; X-ray diffraction; microstructure; dielectric properties
4. Description Abstract

Single-phase (1 – x)(K0.5Na0.5)NbO3⋅xBaZrO3 (x = 0–0.06) ceramics with new compositions, including those modified with SiO2 and ZnO oxide additions, have been prepared and their crystal structure, microstructure, and dielectric and nonlinear optical properties have been studied. A phase with the perovskite structure and an orthorhombic unit cell has been shown to form in all of the synthesized materials. Partial replacement of cations of the basic composition by cations of the combined additive has been demonstrated to cause an increase in unit-cell volume. The ferroelectric phase transitions in the ceramics have been confirmed by dielectric spectroscopy and laser radiation second harmonic generation measurements. Doping with SiO2 and ZnO oxide additions has been shown to lower the temperatures of the transitions from the orthorhombic ferroelectric phase to a tetragonal ferroelectric one and then to a cubic paraelectric phase.

5. Publisher Organizing agency, location The Russian Academy of Sciences
6. Contributor Sponsor(s)
7. Date (DD-MM-YYYY) 01.02.2023
8. Type Status & genre Peer-reviewed Article
8. Type Type Unknown
9. Format File format
10. Identifier Uniform Resource Identifier https://ogarev-online.ru/0002-337X/article/view/140137
10. Identifier Digital Object Identifier (DOI) 10.31857/S0002337X23020082
10. Identifier eLIBRARY Document Number (EDN) YDIQVI
11. Source Title; vol., no. (year) Inorganic Materials; Vol 59, No 2 (2023)
12. Language English=en
13. Relation Supp. Files (48KB)
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14. Coverage Geo-spatial location, chronological period, research sample (gender, age, etc.)
15. Rights Copyright and permissions Copyright (c) 2023 Г.М. Калева, Е.Д. Политова, С.А. Иванов, А.В. Мосунов, С.Ю. Стефанович, Н.В. Садовская